大气降尘对土壤主要环境元素的累积影响及评价——以山东省高密市为例

doi:10.11720/wtyht.2024.1136

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Abstract

This study aims to investigate the pollution distribution of major environmental elements of atmospheric dust fall in Gaomi City, Shandong Province, as well as its effects on soils in a supergene environment. Hence, this study systematically collected and tested the atmospheric dust fall from Gaomi City, obtaining the testing data of nine environmental elements, including Cu, Pb, Zn, Ni, Cr, Cd, As, Hg, and Se. Furthermore, this study calculated the annual sediment fluxes and annual increments of these elements, simulated the minimum annual sediment fluxes for them to reach limit values, and evaluated their pollution levels. The results show that the average contents of various elements in atmospheric dust fall all exceeded their soil background values, exhibiting different degrees of enrichment. In terms of annual sediment fluxes, Cu was significantly positively correlated with Pb, while Zn, Ni, Cr, Cd, As, and Hg were mostly positively correlated in pairs, and Se showed a non-significant correlation with other elements. A higher correlation suggests a higher homology. Atmospheric dust fall, serving as an input end member of major environmental elements in soils, resulted in annual growth rates of various elements in topsoils ranging from 0.03%~0.52%. Cd would be the closest to its soil limit value over a few years. As revealed by geoaccumulation index-based evaluation, Ni, As, and Cr exhibited non-pollution to slight pollution, Se primarily manifested heavy pollution, Cd and Zn displayed moderate to heavy pollution, and Hg, Cu, and Pb mainly showed slight to moderate pollution, corresponding to a pollution order of Se>Cd>Zn>Hg>Cu>Pb>Ni>As>Cr.

Key words： atmospheric dust fall environmental element annual sediment flux annual increment geoaccumulation index

Received: 24 March 2023 Published: 26 February 2024

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	Bing JIANG
	De-Ming ZHANG
	Yang LIU

Cite this article:

Bing JIANG,De-Ming ZHANG,Yang LIU. Cumulative effects of atmospheric dust fall on major environmental elements in soils and their evaluation: A case study of Gaomi City, Shandong Province, China[J]. Geophysical and Geochemical Exploration, 2024, 48(1): 228-236.

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https://www.wutanyuhuatan.com/EN/10.11720/wtyht.2024.1136 OR https://www.wutanyuhuatan.com/EN/Y2024/V48/I1/228

Sampling sites of the study area

Statistical parameters of main environmental elements in atmospheric dust fall 10^-6

Annual sedimentation flux of main environmental elements mg·(m²·a)^-1

Rotational load of main factor

Correlation analysis of annual sedimentation fluxes for main environmental elements

Spatial distribution of annual sedimentation fluxes for main environmental elements

Annual increment of main environmental elements in topsoil caused by atmospheric dust fall μg·(kg·a)^-1

Minimum annual sedimentation fluxes required to reach the limit value and its comparison with the current annual sedimentation fluxes

Box diagram of geoaccumulation index for main enviromental elements

Spatial distribution of geoaccumulation index for main enviroment elements

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